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Electrochemical monitoring of steel corrosion in NS4 solution under cathodic protection environment : insights of electrochemical impedance spectroscopy
Journal article   Open access   Peer reviewed

Electrochemical monitoring of steel corrosion in NS4 solution under cathodic protection environment : insights of electrochemical impedance spectroscopy

Mandlenkosi George Robert Mahlobo, Tumelo Wordsworth Poloko Seadira, Major Melusi Mabuza and Peter Apata Olubambi
Materials and corrosion, Vol.77(7), pp.1159-1166
07/2026
Handle:
https://hdl.handle.net/10210/520202

Abstract

cathodic protection electrochemical impedance spectroscopy mild steel scanning electron microscope simulated soil solution x‐ray diffraction
Effective techniques are crucial for enhancing the durability of underground steel pipelines. Cathodic protection (CP) is commonly used to prevent corrosion, but long‐term monitoring is limited by intrusive methods. This study evaluates electrochemical impedance spectroscopy (EIS) to track corrosion product formation on steel exposed to a soil‐mimicking solution under CP. The steel was immersed for 15 days, with CP applied for 11 days, and EIS measurements recorded periodically. Voltammetric measurements showed that CP reduced the corrosion rate from 410 to 7 µm yr⁻¹ between days 5 and 15. EIS results indicate that, under open circuit conditions, the electrochemical response is consistent with mixed activation–diffusion behavior, whereas under CP the impedance response becomes dominated by activation and interfacial film effects within the measured frequency range. This shift is associated with substantial modification of the interfacial environment and the development of a more resistive surface film. X‐ray diffraction identified the formation of calcareous deposits, primarily aragonite and brucite, together with iron oxide corrosion products. Electrochemical impedance spectroscopy (EIS) monitored corrosion on mild steel under cathodic protection in soil‐like conditions. CP reduced corrosion from 410 to 7 µm/yr, shifting the mechanism from mixed activation–diffusion to activation‐controlled, enabling protective calcareous and oxide film formation.
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https://doi.org/10.1002/maco.70137View
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